Computational Modeling of Protective Clothing
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1 ORIGINAL PAPER/PEER-REVIEWED Computational Modeling of Protective Clothing By James J. Barry, Principal Engineer, and Roger W. Hill, Engineer, Creare Inc. ABSTRACT Models based on computational fluid dynamics (CFD) have been developed to predict the performance of chemical and steam/fire protective clothing. The software computes the diffusive and convective transport of heat and gases/vapors; capillary transport of liquids; vapor and liquid sorption phenomena and phase change; and the variable properties of the various clothing layers. It can also model the effects of sweating and humidity transport to help assess the thermal stress imposed on the wearer of the clothing. Specialized geometry/grid representations of clothed humans have been created for performing two- and three-dimensional simulations. Comparisons with experimental data show good agreement in predicting the effects of fiber swell due to transients in humidity, and the models have been used to predict the sensitivity of clothing performance to material properties such as permeability under varying environmental conditions. Applications of the models include analysis of chemical protective garment design for military and emergency response personnel, comparisons of thermally protective materials for steam or fire protection, and evaluation of clothing test data. NOMENCLATURE c p constant pressure specific heat (J/kg-K) h enthalpy (J/kg) h v enthalpy of vaporization (J/kg) J species diffusion flux (kg/m 2 -s) k eff effective thermal conductivity (W/m-K) K intrinsic permeability (m 2 ) m mass fraction m m mass source per unit volume (kg/m 3 -sec) Q enthalpy of desorption from solid phase (J/kg) p pressure (N/m 2 ) P c capillary pressure (N/m 2 ) R fiber regain (kg bw /kg ds ) S source term s saturation t time (s) T temperature (K) v velocity (m/s) GREEK SYMBOLS ε volume fraction (m 3 of quantity/m 3 ) µ dynamic viscosity (N-s/m 3 ) ρ density (kg of quantity/m 3 of quantity) SUBSCRIPTS β liquid-phase γ gas phase σ solid phase bl bound liquid ds dry solid lv liquid-to-vapor ls liquid-to-solid sat saturation sv solid-to-vapor v vapor INTRODUCTION Protective clothing provides laboratory and hazardous materials workers, fire fighters, military personnel, and others with the means to control their exposure to chemicals, biological materials, and heat sources. Depending on the specific application, the textile materials used in protective clothing must provide high performance in a number of areas, including impermeability to hazardous chemicals, breathability, 25 INJ Fall 2003
2 light weight, low cost, and ruggedness. Nonwoven textiles provide key components of an increasing number of these protective garments. Development of protective materials presently relies heavily on testing. Swatches of textile materials undergo laboratory tests to measure their properties, and the performance of partial or complete clothing products are measured in test chambers or field tests. The objective of the work reported here is development of computational models for predicting the performance of textile materials in protective applications. Such models complement testing by enabling property data from tests of textile swatches to be used in predictions of integrated multilayer garments under varying environmental conditions. Computational fluid dynamics (CFD) provides the basis for the models. In CFD, software solves the governing equations for mass, momentum, and heat trans- TRANSPORT AND PHASE CHANGE PROCESSES IN Figure 1 fer in fluids over a two- or three-dimensional computational mesh. The calculations result in predictions of FABRIC MODEL the flow velocity, temperature, pressure, and composition at each location in the mesh. Though commercial CFD software provides many built-in capabilities, it does not offer (1b) all of the physical models required to address the complex multiphase processes that occur in textile fabrics. As Vapor continuity equation: described in this paper, detailed models for these processes have been developed, integrated into widely used commercial (2a) software, and used for a series of validation and applications calculations. FABRIC MODEL FORMULATION The fabric model simulates the transport of a liquid- and vapor-phase fluid that can undergo phase change (e.g., water) and an inert gas (air) in a textile layer, as illustrated in Figure 1. Several new models and capabilities were added to a standard commercial CFD code (FLUENT Version 6.0, Fluent Inc., Lebanon, NH). These capabilities include: Vapor phase transport (variable permeability) Liquid phase transport (wicking) Fabric property dependence on moisture content Vapor/liquid phase change (evaporation/condensation) Sorption to fabric fibers In the fabric, transport equations are derived for mass, momentum, and energy in the gas and liquid phases by volume-averaging techniques (Gibson; 1994, 1996). Definitions for intrinsic phase average, global phase average, and spatial average for porous media are those given by Whitaker (1977, 1998). Since the fabric porosity is not constant due to changing amounts of liquid and bound water, the source term for each transport equation includes quantities that arise due to the variable porosity. These equations are summarized in general form below. Gas phase continuity equation: (1a) Gas phase momentum equation: Liquid transport: (2b) (2c) (3a) (3b) (4a) (4b) 26 INJ Fall 2003
3 Energy equation (combined): (5a) The model equations are recast into a form compatible with the base CFD code, then implemented using the software s user-defined function (UDF) capability. An extension to the CFD software s graphical user interface (GUI) provides the means to adjust fabric parameters. Figure 2 illustrates the integration of the models with the CFD software. (5c) In addition to the transport equations, a substantial body of supporting equations for properties and interphase exchange rates are included. Permeability is estimated using experimentally determined permeabilities at dry and saturated conditions assuming that the flow resistance is proportional to the regain: Relative permeability constitutive relationships are based on saturation (Wang and Beckerman, 1993; Perre et. al., 1993). Effective thermal conductivity is computed by the method of Progelhof et al. (1976). Capillary pressure is represented by the Leverett J-function form (Udell, 1984; Wang and Beckerman, 1993). Figure 2 INTEGRATION OF FABRIC MODELS WITH CFD SOFTWARE (6) MULTIDIMENSIONAL REPRESENTATIONS OF CLOTHED HUMANS To simulate clothing performance, computational representations of clothed humans have been developed using geometry and grid generation tools. To elucidate the basic physics, a simple 2-D cylinder sized to mimic a human arm is clothed with one or more layers of fabric, Figure 3. The fabric layers may vary in number, thickness, and concentricity. The relatively small size of the mesh (about 14,000 cells) enables calculations to be completed quickly, allowing for significant numbers of sensitivity runs. Figures 4 and 5 depict more complex 3-D models of an arm and torso, respectively. Two layers of fabric clothe the arm. The undulations visible on the clothing surface near the inner elbow are in the outer layer of fabric only. The torso model here is clad in a single fabric layer, a crew-neck T-shirt. Both (5b) Figure 3 2-D MODEL OF A SIMPLIFIED ARM: (A) WITH UNIFORM GAP AND TWO CLOTHING LAYERS; (B) GEOMETRY WITH SINGLE CLOTHING LAYER AND NONUNIFORM GAP 27 INJ Fall 2003
4 Figure 4 3-D MODEL OF ARM WITH TWO CLOTHING LAYERS Figure 5 3-D MODEL OF TORSO (CLAD IN T-SHIRT) arm and torso models are based on laser scans of humans. Scanned points are brought into computer-aided design software for creation of the body surface and generation of clothing layers. The geometry is then exported to the CFD software s preprocessor for grid generation. The arm and torso models have approximately 0.2 million and 1.2 million grid points, respectively. Figure 6 illustrates a 3-D representation of a soldier. This representation models only flow over the outer surface of the clothing and protective gear rather than the heat and mass transfer within the fabrics themselves. Its primary purpose is predicting the flow field immediately around the soldier (including recirculation zones downstream) for assessing impingement of wind-driven chemical agents. This computational representation was developed from a commercial Viewpoint Premier 3-D digital image that was imported into Figure 6 3-D MODEL OF KNEELING SOLDIER IN PROTECTIVE GEAR the CFD grid generation software for simplification (i.e., removal of excessive detail), creation of an enclosed volume, and meshing. The resulting computational mesh uses approximately 1.6 million grid points. COMPUTATIONAL RESULTS Using the gridded human representations and the CFD software with integrated fabric physics models, a wide range of calculations can be performed. The sections below give several illustrative examples, including some validation comparisons with experimental data. Steady-State Data Comparison for Dynamic Moisture Permeation Cell. A single piece of a cotton fabric sample 28 INJ Fall 2003
5 Relative humidity at the bottom outlet Table 1 SEQUENCE OF CHANGES IN RELATIVE HUMIDITY FOR DMPC TRANSIENTS State Initial Condition Transient 1 Transient 2 Transient 3 Transient 4 Inlet Flow Relative Humidity 0% above and below 100% above and below 0% above and below 60% above, 0% below 80% above, 0% below Figure 7 RELATIVE HUMIDITY AT THE DMPC LOWER CHANNEL EXIT (CENTER) VERSUS PRESSURE DIFFERENCE BETWEEN THE UPPER AND LOWER CHANNELS (0.384 mm thick) is placed in the center of an experimental apparatus known as the DMPC (Dynamic Moisture Permeation Cell) described in Gibson (1996) and Gibson et al. (1995). In this cell, a small rectangular swatch of fabric is clamped in place, and controlled flows of gas and/or vapor flow parallel to its upper and lower surfaces. For the data considered here, inlet nitrogen flows at 0.57 m/s above and below the sample. The upper flow is at 100% relative humidity, while the lower flow is at 0% relative humidity. Pressures in the upper and lower flow streams are set to impose a pressure difference across the sample, so that gas is forced through the fabric. Figure 7 provides a plot of the relative humidity at the bottom outlet as a function of the pressure difference across the fabric sample. Positive P indicates a condition where a higher percentage of flow leaves the lower channel exit. Numerical results are provided for three cases: the fabric layer thickness discretized with one, two, or eight cells. All sets of the computed results follow the experimental data trend with pressure drop closely. The minor deviations from the experimental data are attributed to possible small differences between the modeling input parameters and the experimental conditions, actual fabric flow resistance that is not linearly proportional to the fabric regain, and fabric regain that deviates from the assumed regain function with relative humidity. The ability to obtain accurate results even for very coarse discretizations of the fabric is important, since fine discretizations can make large 3-D simulations impractically expensive to perform. Transient Data Comparisons for Dynamic Moisture Permeation Cell. Also using a model of a DMPC, comparisons were made of the predicted temperature response in the center of the fabric samples with transient DMPC experimental thermocouple measurements. In these tests, the DMPC was loaded with two layers of a given fabric (cotton, nylon, silk, polyester, or wool) with a thermocouple located between the layers to record temperature. In the cases considered here, inlet flow rates of 0.57 m/s of nitrogen at 20ºC are again supplied above and below the fabric samples. The humidity of the inlet flows is varied with time to provide transient conditions. Starting at t = 0 sec, the system undergoes a series of four step changes in the relative humidity of the inlet flows as shown in Table 1. The switches in relative humidity occur at 30-minute intervals (15 minutes for polyester). Increases in the relative humidity induce sorption of water from the moist N 2 into the dry fibers and a release of the latent heat and heat of sorption as the fibers approach equilibrium with relative humidity conditions of the incoming gas. Decreases in relative humidity induce desorption of the bound water which requires thermal energy to supply the latent heat and heat of sorption. (Note that for these transients no free liquid is present.) Consequently, step increases in relative humidity produce an initial rise in fabric temperature while step decreases produce an initial fall in fabric temperature. An effective diffusion coefficient for absorption of moisture into the fabric fiber was determined by fitting to data for the first peak in humidity (Transient 1) and used without change for the full transient calculation. Figure 8 compares predicted temperatures with the DMPC experimental data for cotton, nylon, silk, polyester, and wool. The magnitude and trends of the simulated temperatures agree well with the experimental data for all of the materials and inlet condition step changes. The largest deviations between model and experiment are seen for large humidity changes for wool, where the relaxation of the temperature back after the sorption-induced spike is slower in the simulations. Flow Over 2-D Arm Clothed in Nonwoven Material. Simulations were performed using the 2-D model of a simplified arm shown in Figure 3a using a single protective clothing layer of 130 µm thick Tyvek. The layer was placed such that a 1.1 cm uniform gap was present between the arm and the Tyvek inner surface. The Tyvek was assumed to have a permeability of 1.52x10-14 m 2 based on experimental air permeability measurements. From water vapor permeability data, the diffusion coefficient for vapor transport through the Tyvek layer was estimated to be 300 times smaller than for diffusion 29 INJ Fall 2003
6 Figure 8 COMPARISON OF SIMULATED AND EXPERIMENTAL TEMPERATURES FOR VARIOUS CLOTH SAMPLES IN THE DMPC of water vapor in air. Simulations were performed as transients, with initial conditions of a temperature of 300 K and humidity of zero. At the beginning of the transient, a 2.5 mph dry wind was imposed on the system. To mimic conditions of a resting metabolic load, a sweat flux of 1.5x10-5 kg/m 2 and heat flux of 60 W/m 2 was applied at the surface of the arm. For this simulation, thermal radiation was included since it is the dominant mode of heat transfer in the gap between the arm and the clothing material due to the low permeability of Tyvek. Figure 9 shows the contours of temperature at 5, 25, and 75 seconds into the transient. Contours of the water vapor mass fraction are shown in Figure 10 for the same times. The surface of the arm is observed to quickly reach a temperature of about 303 K. The evaporation of sweat increases the water vapor mass fraction in the gap layer at a constant rate until the air becomes saturated at the arm surface at a time of about 22 seconds. After this time, the sweat flux and heat flux remain the same, but a decreasing amount of the sweat evaporates (the balance accumulates as liquid on the skin surface) causing the temperature at the arm surface to rise until it reaches a temperature of about 308 K. (Note that the water vapor mass fraction plots use a log scale to enhance visualization of the concentration outside the fabric layer. The flow structure observed to the right of the cylinders is due to the vortex shedding.) A fabric with a lower resistance to air flow through the fabric or vapor diffusion through the fabric would result in a lower equilibrium temperature. 3-D Model of Human Torso. Figure 11 illustrates a simple example of heat transfer from a 3-D model of a human torso. Using the computational mesh of Figure 5, a 5 mph wind at 300K and 70% relative humidity is imposed on the front of the torso, with skin conditions set to reflect a moderate workload: a sweat flux of 3x10-5 kg/m 2 -s and heat flux of 100 W/m 2. The 30 INJ Fall 2003
7 Figure 9 TEMPERATURE CONTOURS FOR FLOW OVER A SIMPLIFIED 2-D ARM WITH A SINGLE PROTECTIVE LAYER Figure 10 WATER VAPOR MASS FRACTION CONTOURS FOR FLOW OVER A SIMPLIFIED 2- D ARM WITH A SINGLE PROTECTIVE LAYER T-shirt is modeled as 1 mm thick cotton fabric. Figure 11a shows the temperature at the skin surface and velocity vectors in a plane around the torso for conditions of full closure between the layer of clothing and skin at the bottom of the shirt, ends of the sleeves, and at the neck (i.e., snug fit at neck, sleeves, and waist). Figure 11b and 11c show the temperature at a slice slightly below the armpit for the same conditions and for conditions wherein the closures are open (i.e., loose fit at neck, sleeves, and waist). As shown in the figures, the highest temperatures are under the arm. Furthermore, the presence of the closures and their effect of limiting the ability of flow from the environment to enter the area under the shirt results in higher temperatures (as expected). Protection From Chemical Agents. The simplified twodimensional model of an arm (Figure 3) has been used to explore in detail the variation of agent exposure at the arm to variables such as wind speed, location of the liquid droplet on the clothing surface, and gaps between clothing and skin. The evaporation and transport of vapor from a liquid agent droplet on a clothing surface is modeled as a small region of the clothing with sufficient liquid agent present such that the 31 INJ Fall 2003
8 Figure 12 SCHEMATIC OF BASE GEOMETRY FOR TWO-DIMENSIONAL SIMULATIONS OF EVAPORATING SURFACE AGENT (WITH DROPLET LOCATIONS SHOWN) Figure 11 SIMULATION RESULTS OF CLOTHED 3-D HUMAN TORSO: (A) TEMPERATURES AT SKIN SURFACE AND FLOW AROUND TORSO WITH COMPLETE CLOSURE (SNUG FIT) AT NECK, SLEEVES, AND WAIST; (B) TEMPERATURE NEAR ARM PIT FOR COMPLETE CLOSURE; (C) TEMPERATURE NEAR ARM PIT FOR OPEN CONDITIONS (LOOSE FIT) AT NECK, SLEEVES, AND WAIST. air in this region remains saturated with agent vapor (as determined by the vapor pressure of the liquid agent). Transport of the liquid agent itself is neglected (i.e., it cannot wick and does not occupy volume) and the system is assumed isothermal. This simplified approach models agent vapor carried away by the flow over and through the clothing layer but does not track the rate of evaporation or time to dissipate a droplet of known size. Figure 12 shows the base geometry: a 10 cm diameter arm covered with a single 0.5 mm thick clothing layer having a 1.1 cm gap between the surface of the arm and the clothing layer. Fabric permeability was assumed to be a cotton shell (permeability approximately 2.4x10-12 m 2 ) without chemical absorbent materials. Vapor properties correspond to GB (Sarin). The transient simulations were performed with a time step chosen to resolve the shedding frequency of the familiar von Karman vortex street for flow over a circular cylinder. Two wind speeds (5 and 20 mph) were simulated. The following sets of geometric parameters were considered: Base Geometry with an incident wind direction of 0 o, 45 o, 90 o, 135 o, and 180 o relative to droplet. Condition of 0 o corresponds to droplet located at stagnation point. Wind direction at 0 o relative to droplet with single clothing layer having uniform gap spacings of 0.2, 0.6, 1.1, and 2.1 cm. Wind direction at 0 o relative to droplet with single clothing layer eccentric to the arm with non-uniform gap spacing of 4.1:1, and 6.8:1 (maximum/minimum of cm/0.433 cm
9 Agent Concentration (mg/cm 3 ) Figure 13 AVERAGE AGENT CONCENTRATIONS AT THE SKIN (BASELINE GEOMETRY) AS FUNCTIONS OF WIND SPEED AND AGENT DROPLET LOCATIONS and cm/0.282 cm, respectively with minimum thickness located at the stagnation point). The 4.1:1 geometry is shown in Figure 3b. Wind direction at 0 o relative to droplet with two clothing layers (Figure 3a) having uniform gap spacings. First case with inner surface of inner and outer layers located 0.55 cm and 1.1 cm from arm surface, respectively. Second case with inner surface of inner and outer layers located 1.1 cm and 2.1 cm from arm surface, respectively. All simulations were run until the air flow reached a stationary oscillatory state. Agent concentration was assessed to determine the maximum concentration and the area-averaged concentration over the arm surface. The results of the simulations indicate that the predicted agent exposure depends on a competition between penetration of agent through the clothing (which causes higher exposure) and dilution of agent vapor (higher air penetration reduces exposure concentrations). Specific observations include: Agent droplets located at the stagnation point result in the highest exposures. At 5 mph wind speed, diffusion remains a major transport mechanism under the clothing. Agent exposures are the same order of magnitude for all orientations. The stagnation point orientation, i.e., 0 o, gives 2 to 3 times higher exposures than the other orientations. For 20 mph wind speeds, convection becomes more dominant, and dilution becomes a significant effect. Resulting exposures are one to two orders of magnitude lower than for 5 mph for all orientations except 0 o (stagnation point). At the stagnation point, exposures increase at high wind speeds. Increasing gap width and multiple clothing layers have a 33 INJ Fall 2003 relatively small effect on agent exposure for droplets located at the stagnation point. Reduction of the gap near the droplet, however, can significantly increase exposure. Figure 13 illustrates these results for the baseline geometry. The average concentration of agent at the skin surface is highest when the agent droplet is located at the stagnation point, and higher wind speeds enhance this effect. When droplets are located elsewhere, however, the increase in dilution caused by the higher wind speeds reduces the average concentration. Liquid Wicking in a Nonwoven Wipe. A thermally bonded composite nonwoven material of 70% polypropylene and 30% cellulose was used in numerical simulations of a simple wicking experiment. In the experiment, the material was suspended vertically and lowered until the bottom edge was submerged in a pool of liquid water at approximately 20 C. The water immediately began to wick upward into the sample, and the process was recorded on videotape for subsequent extraction of the wicking height as a function of time. Figure 13 shows the experimentally observed liquid height in the sample above the free surface of the liquid as a function of time. The experiment was repeated four times with different samples with no significant difference observed in the wicking behavior. To perform the computational simulations of these tests, several key material properties that characterize the nonwoven sample were needed. Sample thickness measurements along with air flow and pressure drop measurements through a sample were used to determine the intrinsic permeability. Absorption of water into the bound state was neglected, a very reasonable assumption for the polypropylene fibers but an area for refinement in treatment of the cellulose fibers, especially for more accurate treatment of long-time behavior. The porosity was estimated (not measured) to be 70% for the calculations. The gas and liquid relative permeabilities were assumed to be third order functions of the relative saturation. The computational domain included both the vertical nonwoven sample and an adjacent gas region over which a very low velocity saturated and isothermal air flow was forced (resulting in negligible evaporation effects). At t = 0s, a liquid saturation, s, of 0.99 was imposed at one end of the composite sample in which an irreducible saturation of 0.1 was assumed, and the transport equations (excluding the energy equation) were integrated in time. (The liquid saturation is defined as the ratio of the liquid volume fraction to the sum of the liquid and gas volume fractions.) Figure 14 shows the liquid height as a function of time for two cases (the height was defined as the location where the liquid saturation was approximately equal to the irreducible saturation). Given uncertainties in the nonwoven properties,
10 Wicking Height Figure 14 LIQUID HEIGHT VS. TIME FOR WATER WICKING VERTICALLY INTO A NONWOVEN COMPOSITE the numerical simulations show very good agreement with the experimental observations. The simulation assuming a capillary pressure function based on 100% of the water surface tension value overpredicts the wicking height. However, decreasing the capillary pressure function by a factor of two brings the numerical solution into much closer agreement. The reduction is capillary pressure function could be interpreted as the presence of a non-zero contact angle in the composite, a plausible situation considering that the material is 70% polypropylene and initially dry. CONCLUSION In the development of protective clothing and other textiles, modeling offers a powerful companion to experiments and testing. Detailed models for vapor and liquid phase transport within textile fabrics have been developed and integrated with CFD software. Validation of the models with experimental data has been successful for moisture absorption, permeability, and wicking. Validation with additional data for more varied conditions is needed. Applications of the software thus far have included analysis of chemical penetration of garments due to wind, investigation of flow in swatch-testing equipment, and effects of seal leakage on protective clothing performance. Future applications could involve assessment of thermal comfort/stress on wearers of protective clothing, effects of layering on protective performance, and sensitivity to textile permeability and wicking properties. New opportunities for validation and application of the modeling tools are sought. ACKNOWLEDGEMENTS This work was supported by the U.S. Army Soldier Biological Chemical Command under contract DAAD16-00-C References P.W. Gibson, Governing Equations for Multiphase Heat and Mass Transfer in Hygroscopic Porous Media with Applications to Clothing Materials, Technical Report Natick/TR-95/004 (U.S. Army Natick Research, Development, and Engineering Center, Natick, MA, 1994). Gibson, P. W., Multiphase Heat and Mass Transfer Through Hygroscopic Porous Media with Applications to Clothing Materials, Technical Report Natick/TR- 97/005, U.S. Army Natick Research, Development and Engineering Center, Natick, MA, Gibson, P. W., Kendrick, C., Rivin, D., Sicuranza, L., Charmchi, M., An Automated Water Vapor Diffusion Test Method for Fabrics, Laminates, and Films, Journal of Coated Fabrics, Vol. 24, 1995, pp Perre, P., Moser, M., and Martin, M., Advances in Transport Phenomena During Convective Drying with Superheated Steam and Moist Air, International Journal of Heat and Mass Transfer, Vol. 36, 1993, pp Progelhof, R., Throne, J., Ruetsch, R., Methods for Predicting the Thermal Conductivity of Composite Systems: A Review, Polymer Engineering and Science, Vol. 16, 1976, pp Udell, K. S., Heat Transfer in Porous Media Considering Phase Change and Capillarity The Heat Pipe Effect, International Journal of Heat and Mass Transfer, Vol. 28, 1984, pp Wang, C. Y. and Beckerman, C., A Two-Phase Mixture Model of Liquid-Gas Flow and Heat Transfer in Capillary Porous Media I. Formulation, International Journal of Heat and Mass Transfer, Vol. 36, pp , S. Whitaker, in Advances in Heat Transfer, Vol. 13, edited by J. Hartnett, (Academic Press, New York, 1977) p S. Whitaker, in Advances in Heat Transfer, Vol. 31, edited by J. Hartnett, (Academic Press, New York, 1998) p. 1. INJ 34 INJ Fall 2003
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