Development of technologies for the processing and disposal of radioactive waste

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Development of technologies for the processing and disposal of radioactive waste International Experts' Symposium on the Decommissioning of TEPCO's Fukushima Daiichi Nuclear Power Plant Unit 1-41 March 14, 2012 Tokyo, Japan Tokyo Electric Power Company, Inc.

Outline Feature of radioactive waste in Fukushima Daiichi NPP Highly contaminated debris by hydrogen explosions Secondary waste by treatment of contaminated water (zeolite waste, sludge, etc.) We will need to study of properties evaluate for long-term storage develop new technologies for the processing and disposal Introduction of the R&D plan and the its progress

1. Radioactive waste in Fukushima Daiichi Nuclear Power Station

Characteristics of the waste after the accident Influence of injected sea water Sea water affect disposal, corrosion Influence of injected chemicals to protect corrosion Influence of injected boron, etc. Boron affect the environment (consider when disposal) A great variety of radioactive waste Radioactive materials were carried by hydrogen explosions Non radioactive waste change into radioactive waste Influence of core melt down Nuclides originated fuel distributed various place in plant All waste is treated as trans-uranium waste?? R&D consider these characteristics

Example of radioactive waste Scene Waste Dose rate [msv/h] Volume of the waste Treatment for contaminated water Sludge Zeolite Concentrated liquid waste Approx 10 3 Approx 10 1 surface Approx 10 2 at vessel beta ray 581 m 3 346 vessel Approx 105,000 m 3 Actives for plant restoration Debris Logged tree, Soil Liquid waste from decontamination Approx from 10-3 to 10 3 Approx from 10-3 to 10-1 Investigation from now on Approx 34,000 m 3 Approx 59,000 m 3 Dismantling Waste from decommissioning, decontamination Investigation in the future As in the second week of Feb., 2012

Secondary waste produced by the treatment of contaminated water (example) Sludgemade by JAEA Cesium adsorption vessel Tank for concentration liquid waste Zeolite

Debris (example) removal Between Unit 2 and 3 Inside of tent Area of accumulated debris

2. Outline of R&D roadmap towards the disposal

Framework for R&D Planning R&D and progress manegement Research and Development Headquarters will be planning and progress management overall of R&D Working team for radioactive waste processing and disposal ANRE TEPCO JAEA Relevant knowledge and experience, etc. Performing R&D Performing R&D R&D and analysis are performed by JAEA

Outline of R&D roadmap Phase 1 2013 Phase 2 2021 Phase 3 Waste sampling and analysis Revision of R&D plan Holding points Measures for long-term storage decommission waste R&D Using result s Applicability of existing disposal concepts Prospects for disposal Perform and improve the safety of processing and disposal Planning for storage container renewal Establishment for lows, regulations, and technical standard Installation of equipment for production of waste packages Perform the disposal Holding points (HP): The key points for judgment on progression next step HP 8: Verification of applicability of existing concepts HP 9: Verification of prospects for safety

Until HP 8 1. Goals in the near future (from 2012 on) Verification of storage (hydrogen, heat generation) Evaluation for container life Measures for long-term storage Planning for detail of R&D plan 2. Confirm the properties of actual wastes Analysis for few waste (planning) Radioactive, Chemical component, etc. Because of difficulty for actual zeolite sampling, the properties evaluated from result of analysis for treated water. 3. Evaluate for applicability of existing concepts Prospects for disposal for typical waste Identification of problems for typical waste disposal

Until HP 9 1.. Confirm the properties of actual wastes Expand number of results for waste analysis and kinds of waste, Perform actual waste (ex. Zeolite) 2. Solution for problems Problems regarding existing technologies 3. Confirm of prospects for safety 3. Confirm of prospects for safety Compared with the HP 8 Condition of safety evaluation is more detailed Prospects for solution to major problems are verified

After HP 9 1. Establishment for lows, regulations, and technical standard 2. Installation of equipment for production of waste packages 3. R&D for dismantling wastes Confirm the properties of wastes from decommission, decontamination, etc. that produced after HP 9 and R&D for the waste 4. Perform the disposal 4. Perform the disposal Site selection Safety evaluation Waste transportation, etc.

3. Goals in the near future and progress of R&D Secondary waste produced by the treatment of contaminated water

R&D for Secondary waste produced by the treatment of contaminated water Actives for plant restorati on (Outline ) Treatemen t for contamina ted water Storage for secondary waste Development of technologies for processing and disposal of secondary waste produced by the treatment of contaminated water 2012 2013 2014 2015 2016 2017 2018 2019 2020 2021 Existing system Improving the reliability of system Installation of new system Sludge, Zeolite, etc. Confirm the properties Long-term storage Stability storage continued Facility renewal plan Produced waste package Applicability of existing disposal concepts Long-term storage start about 2021 (as needed) Solution for problems

Contaminated water treatment system / Sampling points for radioactive analysis Instead of actual waste sampling, the properties evaluated from result of analysis for treated water Storage tank Sanitization system (Evaporative concentration) Concentra ted waste tank Sanitization system (RO methods) Storage tank Zeolite waste Cesium adsorption apparatus 2nd Cesium adsorption apparatus Decontami nation instruments Sludge We are considering to sampling method for sludge SPT(B) tank Sampling point

Selection for target nuclides on analysis Selected important nuclides for safety evaluation; L1, L2, L3, High level waste, Trans-uranium waste Trench disposal (L3) Concrete, metal, etc. Low level waste Pit disposal (L2) Asphalt- or Cementsolidified product Large-size metal Yoyusindo disposal (L1) Activated metal, resin, Trans-uranium waste, etc. Vitrification, Trans-uranium waste, etc. High level waste Geological disposal Figure of disposal concepts in Japan classified by radioactive level Ground surface 20m 50m 100m 300m over

Flow chart for verification of applicability of existing disposal concept Sludge Debris Logged trees Soils, etc. Results of analysis for wastes Results of analysis for contaminated waters Radioactivity of waste, etc. Evaluation for properties of secondary waste Property of waste package Existing property of waste package Safety evaluation Existing property of disposal technology Holding point Prospects for disposal Problems for processing and disposal Solution for problems

4. Goals in the near future and progress of R&D other waste

R&D for other waste Actives for plant restoration (Outline) Removal of debris from Spent Fuel Pool and upper of Reactor Building (Unit 3) Decontamination of the inside of the Reactor Building Management and strage for radioactive waste Phase 1 Phase 2 2012 2013 2014 2015 2016 2017 2018 2019 2020 2021 Reactor Building SFP Decontamination logged trees, soils Debris from Reactor Building and SFP Decontamination waste Continue Decontamination waste Stability storage continued for debris (Prepare storage area / Dose reduction Stability storage continued for secondary waste produced by treated Facility renewal Change into long-term storage Development of technologies for processing and disposal of radioactive waste In 2012 Confirm the properties Applicability of existing disposal t Solution for problems Development of technologies for and formulation of concepts for processing and disposal of waste Analysis for debris, logged trees, and soils (planning) Planning for detail of R&D plan

5. Challenges for R&D

Challenges 1. Sampling of debris, logged trees Waste grouping method, Number of sample, Typical sample 2. Influence and measure for chlorides If we except chlorides in the waste, how treated with chloride isotopes. Reasonable disposal method for chloride 3. Sampling of zeolite inside of cesium adsorption vessel Because of strong structure and high dose rate, it is difficult to sampling and it is necessary for exclusive instrument to sampling 4. Selection for important nuclides on safety evaluation Especially in this accident, which nuclide we should consider 5. Systematize and prioritize for processing and disposal of a great variety of waste