Impact of traffic composition and street canyon on the street level air quality and pedestrian exposure in Central, Hong Kong

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Impact of traffic composition and street canyon on the street level air quality and pedestrian exposure in Central, Hong Kong Agata Rakowska, Ka Chun Wong, Thomas Townsend, Chan Ka Lok, Dane Westerdahl, Zhi Ning* Aerosol and Air Pollution Group, School of Energy and Environment, City University of Hong Kong Contact: Dr. Zhi Ning; Email: zhi.ning@cityu.edu.hk; Phone: 3442-4620 1. Background Exposure to particulate matter (PM) and nitrogen dioxide (NO2) has been linked with adverse health effects including aggravation of respiratory diseases and reduction in lung function [1]. Vehicle emissions are of the major sources of air pollution in metropolitan cities including Hong Kong. There is an increasing trend around the world with tightening emission control and larger scale of transport policy intervention in urban cities to control the traffic pollutants and reduce public health risks, such as low emission zone and congestion charging etc. In order to investigate the impact of traffic on the roadside air quality and pedestrian exposure, an experimental study was carried out in Central, one of the most developed business districts in Central, Hong Kong. The objectives of the investigation are: To investigate the impact of roadway traffic volume and composition on roadside air quality in Central, especially for busy districts with street canyon effects. To identify the contributing vehicle fleets to the air pollution and pedestrian exposure safety in different streets. 2. Experiment methodology The experiment took place on Wednesday 31 July, Saturday 3 August, Monday 27 October and Sunday 28 October, 2013 covering three very busy streets Connaught Road, Des Voeux Road and Queen s Road showed on the map below in Figure 1. During the measurement campaign, total of 8 sampling periods were successfully conducted in which 6 from weekdays and 2 from weekend. Both street canyon and open roadway configurations were covered in selection of streets. Mobile platform and suitcase based measurement techniques were deployed to monitor both on-road and roadside pollutants concentrations at different time of a day and different days of a week. Multiple traffic counting points were also deployed concurrently to collect the traffic volume and fleet compositions in individual streets, and used to link with the measured pollutants concentrations. Figure 1 Sampling routes and nine traffic counting points. Red dash line is the on-road route and blue solid line is the roadside route. The traffic volume and composition were recorded at nine counting points. 1

Air quality data was collected with two sets of equipment to evaluate both on road street level and roadside pedestrian level pollutant concentrations. One set was the On-road Plume Chasing and Analysis System (OPCAS) that CityU has developed for vehicle emission testing and its route is described as red dash line in Figure 1. The roadside pollutants measurement was performed by Mobile Exposure Measurement System (MEMS), which is a wheel-equipped suitcase configured with portable air monitors and data acquisition system to simulate a pedestrian s exposure to the pollutants while walking along the streets. Additionally, traffic counting was conducted along the three targeted streets: Connaught Road Central (CRC), Des Voeux Road Central (DVRC) and Queen s Road Central (QRC), using the EMFAC 16 Vehicle Classes System (Private cars, motorcycles, taxis, light and heavy goods vehicles, public and private light buses, franchised single and double decker buses and non-franchised buses). A video camera was also synchronized with the same time stamp to ensure the accurate interpretation of the data stream. 3. Results and discussions Traffic pattern Figure 2 shows the weekday traffic volume and fleet composition of CRC, DVRC and QRC streets at different time periods, each representing the average of traffic count from three counting points on the individual street. Consistent traffic pattern was observed on the three streets, in which CRC has the highest hourly total traffic count from 5500 to 7000, while DVRC and QRC have only 550 to 720 vehicles per hour. There was no substantial diurnal variation observed in the traffic volume for all the streets suggesting the typical business district nature of the study area. The dominant fleets in the streets are petrol private car or LPG vehicles Vehicle count per hour 8000 6000 4000 2000 0 Streets and Time Period Figure 2 Traffic volume and fleet composition in the streets during different time periods. (mostly taxi) for CRC (34 to 46%), diesel franchised bus for DVRC (36 to 43%) and petrol car or LPG vehicles for QRC (24 to 46%) as shown in Figure 2. On-road air pollution The traffic related pollutants concentrations of black carbon (BC), PM 2.5, particle number (PN) and NOx showed dramatic difference between different streets. Although CRC has substantially higher total traffic flow, the pollutants concentrations peak at less trafficked street of DVRC, especially for section of CC2 with concentrations of 67.8 (µg/m 3 ), 60273 (#/cc), 53 (µg/m 3 ), 542 (ppbv) for BC, PN, PM 2.5 and NOx, respectively, because of the difference in roadside environments. Previous studies have shown that street canyons in urban areas may trap traffic induced pollutants within their boundaries and increase the pollutant concentrations significantly within the immediate areas around the roadway. Due to the difference in traffic volume, the on- 2 Diesel Buses Diesel Trucks and Vans Petrol Private Cars LPG vehicles Others AM Noon PM AM Noon PM AM Noon PM CRC DVRC QRC

Figure 3 Traffic volume and fleet composition versus street level NOx and black carbon, particle number and PM 2.5 concentration. road pollutants concentrations in the same street also vary. Section CC2 in DVRC has 4.2, 1.8, 1.9 and 1.4 times higher concentrations than section AA2 for BC, PN, PM 2.5 and NOx, respectively. Compared to DVRC with consistent street canyon features, although QRC has similar total traffic volume, the pollutants concentrations were much lower. A further look at the traffic composition shows dominant fleets in DVRC are diesel franchised buses with an average fraction of 39%, followed by petrol and LPG vehicles, while QRC is dominated with LPG and petrol vehicles, each representing 40% and 34%. Our earlier work on the Hong Kong on-road vehicles has shown diesel fleets are the major contributor to the mobile PM emissions especially black carbon, and to a lesser extend for NOx emissions [2]. Additionally, the street canyon in DVRC and QRC significantly restricts the dispersion of traffic emissions. The speed of street level wind during two sampling days, 27 and 28 October, showed the similar pattern in which the wind speeds in DVRC and QRC were substantially reduced compared with QRC. Significant difference in the observed on-road pollutants concentrations is a clear indication of the impact of diesel fleets on the street level air quality and the contribution may be further enhanced by the effect of street canyon. Weekend observations Figure 4 shows the comparison of traffic volume and fleet composition on Sunday and Monday for both morning and noon time periods. The total traffic volume in the morning of Sunday decreased by 45% compared with that of Monday from 9035 to 4970 vehicles/hour due to the Figure 4 Comparison of traffic volume and composition between Sunday, 27th, Oct, 2013 and Monday, 28th, Oct, 2013 for a) Morning and b) Noon periods. 3

regular day-off of the commercial and business activities that lowers the volume of public transport by buses, daily commuting traffic by private cars and commercial goods delivery service with diesel vans and trucks during regular morning rush hours. The traffic pattern during Sunday noon time, however, showed a very different trend, in which the total traffic volume remained almost the same (-4% reduction from Monday to Sunday), while the fleets composition recorded a dramatic change with only volume of commercial diesel vans and trucks decreased by 59% and all other fleets increased by different extent, i.e., diesel bus for 10%, petrol vehicles for 14% and LPG vehicles for 3%, because of increased typical weekend commercial activities in the central business district attracting passenger volume via private and public transport. Figure 5 shows the on-road pollutants concentrations (NO x and BC) measured in different sections of streets and corresponding traffic volume and composition. Significant decrease in traffic volume during Sunday morning period compared with Monday showed consistent trend with the on-road pollutants concentrations with an average reduction of 41%, 40% and 18% for NOx, and 52%, 39% and 36% for BC as measured on CRC, DVRC and QRC respectively. On the other hand, although noon time total traffic volume had only slight change by 4%, the onroad pollutants concentrations recorded a significant reduction on Sunday compared with Monday. Sunday noon time traffic was characterized by increased private and public transport via buses and passenger cars, the documented difference in measured pollutants concentrations is likely due to the less traffic of commercial diesel vans and trucks. Vehicle emissions, being Figure 5 Comparison of weekend (Sunday, 27 Oct, 2013) and weekday (Monday, 28 Oct, 2013) traffic pattern and on-road pollutants concentrations at different time periods: a) Sunday morning; b) Monday morning; c) Sunday noon; d) Monday noon. 4

major source of pollutants in metropolitan cities, have attracted much attention and various policy measures have been implemented worldwide to reduce their impact on urban air quality, for example, congestion charging to passenger cars and low emission zones to limit traffic in city centers [3] with different extent of success [4, 5]. The findings also suggest the potential impact of controlling fleet based vehicles on the improvement of urban air quality. Pedestrian exposure to roadside air pollutants Figure 6 shows on-road and roadside concentrations of black carbon and ultrafine particle number measured in the different streets from the concurrent measurements. Compared to the on-road concentrations, roadside BC and UFP pollutants showed dramatic contrast with ratios of about 50-70% and 90-120% between roadside and corresponding on-road concentrations. The remarkable reduction of BC concentration as evidenced by the roadside to on-road ratios in the study indicates the dilution of exhaust emissions from on-road to roadside environment dominates the dispersion of BC. On the other hand, during dispersion, the exhaust particles may undergo physical and chemical transformation depending on the aerosol dynamical processes, such as condensation, evaporation, nucleation etc. The dramatic difference of the particle number concentration ratio (90-120%) compared with black carbon (50-70%) as observed in this study clearly indicates the role of nucleation in forming ultrafine particles from on-road to roadside. The process may be further enhanced by the street canyon effect in which higher concentrations of traffic emissions of semi-volatile species may be present and contained inside the canyon that facilitate the nucleation formation of ultrafine particles. From the pedestrian exposure point of view, ultrafine particles may pose a greater health risk due to their small size and ability to penetrate deep in the lungs [6]. The result from the present study shows high roadside concentration and ratios with on-road levels by pedestrian exposure inside urban street canyon, where large volume of pedestrian flow often occurs. Figure 6 On-road and roadside pollutants concentrations of BC and ultrafine particles number 4. Conclusion and implication We have identified high association between the volume of diesel fleets and street level pollutants concentrations although they constitute only a fraction of traffic flow, while total traffic volume is not necessarily the driving factor to the air quality. This finding implies traffic control strategy targeting total volume reduction may not be a cost effective approach since small fraction of dirtiest vehicles actually contribute a disproportionally high fraction of total emissions. Given the fact that vehicle emission has become the major pollution sources in urban areas, 5

many governments have implemented local transport policy to improve urban air quality on top of tightening vehicle emission standard, such as low emission zone in European cities [3, 4], congestion pricing in New York [7], restriction of odd/even license of private cars in Beijing [8] etc. The benefits and cost-effectiveness of such transport policies in reducing urban air pollution concentrations need careful evaluation, and relation between pollutant concentrations and traffic volume/flow is the key factor. On the other hand, this study also documented strong street canyon effects and its impact on the increased NO x and BC concentrations and elevated ultrafine particles formation inside streets. Although there is nearly ten times of traffic volume in a wide and open roadway (CRC in this study), its on-road and roadside pollutants showed much lower concentrations than the adjacent streets with canyon effects (DVRC and QRC). The strong contrast observed in the study suggests the necessity of urban air quality management through more integrated urban planning strategy with consideration of their impact on traffic related air pollution and pedestrian exposure to the pollutants. Much more efforts are still needed not only by better understanding the integrated cost-effectiveness, but also by more bureaucratic cooperation in policy making processes. 5. Acknowledgements This study was supported by the Health and Medical Research Fund, Food and Health Bureau, Hong Kong SAR Government (Ref. No. 10112061), and Environmental Conservation Fund, Hong Kong SAR Government (Ref. No. 01/2012). The authors would like to thank the MVA, Hong Kong for their technical support in the traffic information collection and analysis, and Civic Exchange for their support in the implementation of the study. Also the authors thank the team members (in alphabetic sequence) for the assistance of field experiments: Dr. Nirmal Kumar Gali, Mr. Yang Hong, Miss Sabrina Yanan Jiang, Ms. Flora Lau, Miss Li Sun, Miss Viki Wai Ting Tong, Mr. Wubulihairen Maimaitireyimu, Mr. Fenuan Yang. References 1. Saldiva, P.H.N., Air pollution in urban areas: the role of automotive emissions as a public health problem. International Journal of Tuberculosis and Lung Disease, 1998. 2(11): p. 868-868. 2. Ning, Z., M. Wubulihairen, and F.H. Yang, PM, NOx and butane emissions from on-road vehicle fleets in Hong Kong and their implications on emission control policy. Atmospheric Environment, 2012. 61: p. 265-274. 3. Wolff, H. and L. Perry, Trends in Clean Air Legislation in Europe: Particulate Matter and Low Emission Zones. Review of Environmental Economics and Policy, 2010. 4(2): p. 293-308. 4. Boogaard, H., et al., Impact of low emission zones and local traffic policies on ambient air pollution concentrations. Science of the Total Environment, 2012. 435: p. 132-140. 5. Roustan, Y., M. Pausader, and C. Seigneur, Estimating the effect of on-road vehicle emission controls on future air quality in Paris, France. Atmospheric Environment, 2011. 45(37): p. 6828-6836. 6. Oberdorster, G., E. Oberdorster, and J. Oberdorster, Nanotoxicology: An emerging discipline evolving from studies of ultrafine particles. Environmental Health Perspectives, 2005. 113(7): p. 823-839. 7. Schaller, B., New York City s congestion pricing experience and implications for road pricing acceptance in the United States. Transport Policy, 2010. 17(4): p. 266-273. 8. Zhou, Y., et al., The impact of transportation control measures on emission reductions during the 2008 Olympic Games in Beijing, China. Atmospheric Environment, 2010. 44(3): p. 285-293. Note: If you have any questions or comments about the study, please feel free to contact Dr. Zhi Ning from City University of Hong Kong via email: zhining@cityu.edu.hk 6