The DENOPI project: a research program on SFP under loss-of-cooling and loss-of-coolant accident conditions

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The DENOPI project: a research program on SFP under loss-of-cooling and loss-of-coolant accident conditions NAS meeting March 2015 N. Trégourès, H. Mutelle, C. Duriez, S. Tillard IRSN / Nuclear Safety Division / Safety Research

Fukushima Daiichi Unit 4 SFP (OECD Status Report on SFP 2015) On 2011/03/11: 1535/1590 fuel assemblies, 1331 spent fuels, 204 fresh fuels Decay heat: 2.26MWth Time estimation of fuel assembly dry out: end of March 2011 Due to delay in maintenance, the reactor well was filled with water on March 2011 Pressure from the reactor well side as the SFP water level became low induced a water inflow from the reactor well to the pool Intensive water injection conducted between April 22 and 27 Twater ~ 80-90 C during ~4.5 months Recovery of active heat removal on 2011/07/31 @ Twater ~ 75 C On 2011/08/03 -> Twater ~ 40 C 2/12

2013: IRSN launches the DENOPI program within the framework of the «Investment for the future» programs funded by the French Government Scope: Spent Fuel Pool under loss of cooling and loss of coolant accident conditions Safety objectives: - to study the different phases and the timing of the accident, - to assess mitigation strategies, - to assess safety margins. How: - experimental investigations, - computer code analysis. Schedule: 2014-2019 Partners: French academic labs 3/12

IRSN strategy = experimental investigations at three scales A: Thermal hydraulics at the pool scale Loss of cooling - Early phase of the accident C: The clad behavior under airsteam oxidation B: LOCA at the assembly scale Spray efficiency Criticality Air ingress 4/12

A SFP Loss of Cooling - Studies at pool scale (1/2) Objectives: Get an experimental data base on the TH behavior of a SFP in case of a loss of cooling accident before assembly uncovery : - convective loop patterns and intensity? - influence of power distribution in the SFP? Validation of computer code??? Patterns during loss of cooling? (failure of active heat removal system) Experimental devices : Cold water injection Patterns after recovery of active heat removal system To collect experimental data on a pool mock-up at reduced scale for code validation 5/12

A SFP Loss of Cooling - Studies at pool scale (2/2) 3D tests at reduced scale a Supporting calculations - Analysis Dimensionless numbers SFP Mock-up Two possible options Q D T 6,3 10 5 8,3 10 4 7 10 14 1,6 10 12 0,22 0,22 73 70 0,0013 0,014 6/12

B - Studies at assembly scale (1/3) Objectives: 1. To evaluate coolability of uncovered assemblies by water sprays MEDEA facility 2. To evaluate criticality risk (Thermal hydraulic conditions) 3. To get knowledge on two-phase thermal-hydraulic behavior of an assembly for dewatering transients, steady-state conditions with water levels ASPIC facility 4. To evaluate conditions for air penetration into the assembly Dedicated small scale device 7/12

B - Studies at assembly scale (2/3): MEDEA device 1- Flooding studies: 2- Wire mesh sensor qualification (void fraction measurement): Water/air separator Water injection 17*17 unheated rod bundle Transparent walls Air / steam inlet Simulation of various top nozzle geometries Simulation of various water injection systems [0 1 m 3 /h] Flow nozzle (minimal size of bubbles, void distribution, assembly impact on void distribution ) 8/12

B - Studies at assembly scale (3/3): ASPIC device TH behavior of an assembly for dewatering transients, steadystate conditions with water levels, residual powers 12 m 9/12

C - Studies at clad scale (1/2) Objectives: 1. Gain knowledge on the phenomenology of the oxidation process for pre-oxidized cladding in air + steam mixtures to develop a kinetic model that takes into account P O2, P H2O, P N2 for SA code (ASTEC) - how protective is the pre-transient oxide? - effect of steam addition (H-pickup)? 2. Mechanical properties of the cladding after an oxidation transient in air + steam (post-accident handling) : - how brittle are the fuel rods after accidental partial uncovery transient? 10/12

C - Studies at clad scale (2/2) steam partial pressure impact Isothermal oxidation at 850 C Oxidation rate (g m -2 s -1 ) d(dm/s)/dt (g m -2 s -1 ) 0.07 0.06 0.05 0.04 0.03 0.02 0.01 Bare Zy4, oxidation in air Zy4 pre-ox. in O 2 at 425 C (32 µm), oxidation in air Zy4 pre-ox. in autoclave at 360 C (32 µm), oxidation in air Zy4 pre-ox. in O 2 at 425 C (32 µm), oxidation in steam 0 0 60 120 180 240 300 time (min) Time (min) C. Duriez et al. Fontevraud 8 - Avignon 2013, Septembre 14-18 IRSN, unpublished results HT oxidation in air is much faster than in steam, due to formation of ZrN and its oxidation A pre-oxide scale formed at low T delays the air attack at high T. The protective effect depends on the pre-oxidation method. However acceleration due to nitriding still occurs. Addition of steam in the air induces H-pickup during the HT oxidation. H pick-up increases with the steam partial pressure. 11/12

DENOPI Schedule 2014 2015 2016 2017 2018 2019 Feasibility studies Design & fabrication «reduced scale pool» exp. A-Pool scale: Convection loops in a BK pool with uncovered assemblies MEDEA Design & fabrication Exp. plan CCFL tests ASPIC Design & fabrication Air penetration/analytical exp. Assembly scale exp. B-Assembly scale: Air penetration + spray efficiency + TH behavior for LOCA transients Study of O 2 transport in the oxyde layer by RAMAN spectrometry ; in situ DRX O 2 -N 2 -H 2 O impact in the clad degradation process in mixed atmosphère C-Clad scale: Oxidation of fuel in air and steam mixtures + mechanical tests 12/12