INTERNATIONAL WG1-WG4 MEETING on

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European Network on New Sensing Technologies for Air Pollution Control and Environmental Sustainability - EuNetAir COST Action TD1105 INTERNATIONAL WG1-WG4 MEETING on New Sensing Technologies and Methods for Air-Pollution Monitoring European Environment Agency - EEA Copenhagen, Denmark, 3-4 October 2013 Action Start date: 01/07/2012 - Action End date: 30/06/2016 - Year 2: 2013-2014 (Ongoing Action) AIR QUALITY MODELLING IN SLOVENIA: FORECASTING AIR POLLUTION AT REGIONAL AND LOCAL SCALE Rahela Žabkar (MC Member, WG3 Member) University of Ljubljana, Slovenia, Center of Excellence SPACE-SI COST is supported by the EU Framework Programme ESF provides the COST Office through a European Commission contract

Background Why models? - complete spatial coverage of air quality (limited spatial coverage of monitoring) - can be applied prognostically - provide improved uderstanding of the sources, causess and process Model limitations - require extensive input data - due to many uncertainties extensive validations needed - remain a representation of reality 2

Current activities Air quality modelling within meteorology group at University of Ljubljana, Slovenia: Investigating dynamics of air pollution episodes (together with evaluations, verifications of AQ models) Studying feedback effects of aerosols on meteorology (AQMEII initiative, WRF/Chem model) AQ forecasting (WRF/Chem, ALADIN/CAMx, statistical ozone model) Involved in EuNetAir COST Action as member of WG3 (Environmental measurements and air pollution modelling) 3

WRF/Chem forecast Weather Research and Forecast (WRF) model online coupled with chemistry (WRF/Chem) Experimental operational AQ forecast at UL (started in spring 2013) Chemical boundaries (MOZART model) Geographical data (landuse, albedo ) GFSmeteorological initial and boundary conditions WRF/Chem 48 h AQ forecast Center of Excellence SPACE-SI MEGANbiogenic emissions Anthropogenic emissions for EU (TNO/MACC-II) Anthropogenic emissions for SI (national database) 4

WRF/Chem forecast Model version 3.4.1 Two nested domains, horizontal grid spacing (grid points) 11.12 km (151x100) and 3.7 km (181x145) 42 vertical model levels Integration once per day: 00 UTC Integration time 48h Aerosol direct effect included Parameterization schemes: Morrison microphysics, RADM2-MADE/SORGAM, YSU PBL, RRTMG radiation, Noah LSM, G3 cumulus, Fast-J photolysis 5 Available : http://meteo.fmf.uni-lj.si/onesnazenje

ALADIN/CAMx forecast Off-line coupled meteorological (ALADIN) and chemical transport model (CAMx) Running (almost operationally) at Environmental Agency of Slovenia Environmental Agency of Slovenia Chemical boundaries (MOZART model) Additional input fields (landuse, TOMS ) ALADIN/SI meteorological fields CAMx 48 h AQ forecast SMOKEbiogenic emissions Anthropogenic emissions for EU (TNO/MACC-II) Anthropogenic emissions for SI (national database) 6

Statistical ozone forecast 2-day ozone daily maximum forecast at Slovenian Environment Agency for 8 measuring sites Regression type model: meteorological and air quality measurements (yesterday, today early morning), ECMWF forecast for meteorological variables and trajectories at 925 and 850 hpa Important feature: O 3 prediction depends on predicted trajectory cluster (kmeans clustering) Example: Nova Gorica Left: Ozone statistics for trajectory clusters Right: measured / forecasted ozone daily maximum Izračunane urne vrednosti ozona µg/m ( 3 ) 220 180 140 100 60 NGI, 7 skupin 7 60 100 140 180 220 Izmerjene urne vrednosti ozona (µg/m 3 ) St. skupine: 1 2 3 4 5 6 7

Verification of model predictions July & August 2013 - focused especialy on O 3 Measurements from 12 monitoring stations (AirQ; national network) for WRF/Chem forecast (O 3, PM10, SO 2, CO, NOx, NO 2 ) For 8 monitoring stations statistical ozone daily maximum forecast (SF) KOP urban, background NG urban, background OTL rural,background LJ urban, background ISK rural, background KRV rural, background HRA urban, background TRB suburban, background CE urban, background MB urban, traffic MS rural, background 8

ozone (hourly values) - July&August 2013 WRF/Chem: ME: -22 to 28 μg/m 3 ; RMSE: 24 to 40 μg/m 3 ; CORR: 0.48 to 0.71 9

ozone (daily maxima) - July&August 2013 WRF/Chem: ME: -28 to 1μg/m 3 ; RMSE: 9 to 37 μg/m 3 ; CORR: 0.54 to 0.87 Statistical model: ME: -13 to 2 μg/m 3 ; RMSE: 12 to 29 μg/m 3 ; CORR: 0.5 to 0.81 10

ozone (8h maxima) - July&August 2013 WRF/Chem: ME: -26 to 3 μg/m 3 ; RMSE: 12 to 30 μg/m 3 ; CORR: 0.51 to 0.79 11

PM10 (daily values)- July&August 2013 WRF/Chem: ME: -3 (-13) to 6 μg/m 3 ; RMSE: 9 to 18 μg/m 3 ; CORR: 0.23 to 0.49 12

NO2 (hourly values) - July&August 2013 WRF/Chem: ME: -24 to 6 μg/m 3 ; MAE: 5 to 24 μg/m 3 ; RMSE: 8 to 31 μg/m 3 13

Air pollution above the sea Example of 48h forecast for July 24, 2013 Measurements needed to verify model results above the sea 14

Future plans Further model evaluations and verification with additional measurements (spatial, temporal, also stations from neighbouring contries ) Comparison of WRF/Chem forecast with ALADIN/CAMx results Studying the impact that have aerosol feedbacks in coupled model approach on meteorological and AQ forecast (PM concentrations not underestimated as in other studies) Consider possibilities for (off-line) assimilation of measurements to improve AQ forecast 15

Summary of the results and the conclusion WRF/Chem AQ forecast succesfully implemented Generally good (qualitative) agreement between model and measurements Model (quantitative) performance depends on pollutant and station representativness, location O 3 : simulated maxima/minima underestimated/overestimated, bias corrections needed for most (not all) stations, WRF/Chem forecast competitive to statistical model PM10, PM2.5: concentrations almost without bias (!), exception MB urban traffic station To improve model predictions of hourly values (and high pollution episodes) necessary to combine model results with measurements 16

Summary of the results and the conclusion High O 3 levels above the sea explain higher measured O 3 at Mediterranean station in Slovenia Are high PM concentrations above Adriatic realistic, or model artifact? Measurements (AQ, but also meteorological) needed to verify model results above the sea 17

Thank you! rahela.zabkar@fmf.uni-lj.si 18