Characteristics of Modular Fast Reactor SVBR-100 Using Thorium-Uranium (233) Fuel

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Characteristics of Modular Fast Reactor SVBR-100 Using Thorium-Uranium (233) Fuel G.I. Toshinsky ab, O.G. Komlev b, I.V. Tormyshev b, N.N. Novikova b, K.G. Mel nikov b a -JSC AKME-Engineering, Moscow, Russia b -FSUE SSC RF-IPPE, 1, Bondarenkosq., Obninsk, Kaluga rg., 249033, Russia, E-mail: komlev@ippe.ru March 4-7, 2013 FR13, Paris, France 1

1. INTRODUCTION Outline 2. BASIC TECHNICAL CHARACTERISTICS OF RF SVBR-100 3. CORE CHARACTERISTICS WITH URANIUM-THORIUM FUEL OF DIFFERENT TYPES 4. SENSITIVITY OF BREEDING RATIO TO CORE DIMENSIONS AND EXISTENCE OF BREEDING ZONES 5. CORE CHARACTERISTICS WITH URANIUM-THORIUM-PLUTONIUM FUEL 6. CONCLUSIONS March 4-7, 2013 FR13, Paris, France 2

INTRODUCTION 1. Thorium resources in the earth's crust are several times as much as those of uranium (essentially increased raw basis for nuclear power). 2. Technical grounds to use the thorium fuel cycle: thorium-232 is better raw isotope compared with uranium-238 Thorium dioxide is more chemically and radiation resistant Its thermo-physical properties (heat conductivity, linear expansion coefficient) are better less number of plutonium isotopes and long-lived minor actinides is built Nuclide SVBR mean spectrum values σ с, b σ f, b α=σ c /σ f ν f 232 Th 0.30 0.01 29.5 2.01 233 U 0.22 2.46 0.09 2.52 235 U 0.43 1.69 0.26 2.47 238 U 0.26 0.04 6.03 2.44 239 Pu 0.38 1.68 0.23 2.95 inherent supporting of nuclear materials non-proliferation (hard gamma rays emitters bismuth-212, thallium-208) the thorium fuel cycle is preferable for weapon plutonium utilization 3. SVBR RF allows use of various nuclear fuels based on UO2, MOX, UN, (Pu-U)Nand others March 4-7, 2013 FR13, Paris, France 3

BASIC TECHNICAL CHARACTERISTICS OF RI SVBR-100 1. Fast reactor core with chemically inert lead-bismuth coolant (LBC). 2. A monoblock(integral) design of a pool type is used for the primary circuit equipment. 3. A two-circuit scheme of heat removal is used. 4. The levels of coolants' natural circulation in the heat-removal circuits are sufficient to ensure reactor's heat decay removal without over-heating of the core. Parameter Value RF thermal power, MW 280 RF electric power(gross load), MW 101.5 Fuel: type loadof U-235,kg average enrichment in U-235,% UО 2 ~1470 ~16.5 Time between refuelings, years 7-8 Reactor monoblock dimensions(diameter/height), m 4.5/7.5 March 4-7, 2013 FR13, Paris, France 4

CHARACTERISTICS OF U-TH FUEL CYCLE 1. Numerical Model 2. Types of fuel: +, +, + Radiation shielding Reflector Core Reflector Profiling zone number (U+Th) (U+Th)O 2 (U+TH)N Enrichment in uranium-233, % 1 9 10.4 9.3 2 9.6 11.0 9.7 3 10.8 12.4 11.0 4 13.6 15.6 13.2 March 4-7, 2013 FR13, Paris, France 5

CHARACTERISTICS OF U-TH FUEL CYCLE (2) Distribution along the core radius for non-uniformity coefficient of (heated) energy release distribution for nitride fuel (U+Th)N March 4-7, 2013 FR13, Paris, France 6

CHARACTERISTICS OF U-TH FUEL CYCLE (3) Neutron spectra in the core for 3 kinds of fuel March 4-7, 2013 FR13, Paris, France 7

CHARACTERISTICS OF U-TH FUEL CYCLE (4) Fuel type Parameter, dimensionality Metal (U+Th) Oxide (U+Th)O 2 Nitride (U+Th)N Effective fuel density, g/cm 3 10.5 9.6 12.5 Average enrichment in uranium-233, % 11.5 13.2 11.5 Uranium-233 load G 3, t ~1,3 ~1,2 ~1,4 Total load of uranium and thorium G т.а., t ~11,1 ~9,0 ~12,5 Reactivity change over the lifetime, % 8.7 9.1 6.0 U-233 breeding ratio 0.85 0.85 0.9 March 4-7, 2013 FR13, Paris, France 8

SENSITIVITY STUDIES OF URANIUM-233 BREEDING RATIO. BREEDING ZONES Th (fuelpin breeding zone) Th (fuelpin and radial breeding zones) Parameter, dimensionality (U+Th)N Core design + fuelpin breeding + fuelpin and radial zone breeding zones U-233 enrichment, % 11,5 11,6 12,0 Uranium-233 load G 3, t 1,4 1,4 1,5 Total load of U and Th, t 12,5 14,7 21,6 Reactivity change, % 6,0 6,2 6,1 U-233 breeding ratio 0,9 0,92 0,97 March 4-7, 2013 FR13, Paris, France 9

SENSITIVITY STUDIES OF URANIUM-233 BREEDING RATIO. CORE DIMENSIONS Core design Parameter, dimensionality (U+Th)N Core Height is increased by 10cm Core Height is increased by 20cm, Core diameter is increased by ~ 7 cm Average fuel enrichment in uranium-233, % 11,5 10,8 9,7 Uranium-233 load G 3, t 1,4 1,5 1,7 Total load of uranium and thorium, t Reactivity change over the lifetime, % 12,5 13,7 16,6 6,0 4,8 3,2 U-233 breeding ratio 0,9 0,94 0,96 March 4-7, 2013 FR13, Paris, France 10

CHARACTERISTICS OF U-Th-Pu FUEL CYCLE 1. Nitride fuel composition (Th+Pu)N. 2. Isotopic content of Pu corresponds to the spent nuclear fuel of reactor WWER. Isotope Content, % Pu-238 1.7 Pu-239 65.3 Pu-240 23.9 Pu-241 3.6 Pu-242 5.6 Reactivity dependences on the lifetime moment March 4-7, 2013 FR13, Paris, France 11

CHARACTERISTICS OF U-Th-Pu FUEL CYCLE (2) Parameter, dimensionality (U+Th)N Fuel type (Th+Pu)N Average fuel enrichment in uranium-233 or Pu, % 11,5 14,6 Load of uranium-233 or Pu, t 1,4 2,0 Total load of the core, t 12,5 12,5 Reactivity change over the lifetime, % -6,0 +2,0 Breeding ratio 0,9 0,98 March 4-7, 2013 FR13, Paris, France 12

CONCLUSIONS The performed computations for three different types of fuel (oxide, nitride and metallic), have revealed that maximum of uranium-233 breeding ratio, which equals to 0.9, is achieved when nitride type of fuel is used Adding breeding zones or increasing of the core dimensions result in increasing uranium-233 breeding ratio (up to BR = 0,97 or BR = 0,96 respectively). There is opportunity of using plutonium as initial fissile isotope to implement U-Th-Pu fuel cycle. Breeding ratio is assessed by 0,98 if nitride fuel composition (Th+Pu)N with effective density of 12.5 is used. The obtained data have demonstrated that both for U-Th FC and U-Th-Pu FC there is an opportunity to achieve a value of U-233 BR to be over unity when using the breeding zones and slightly increased the core dimensions. March 4-7, 2013 FR13, Paris, France 13