Pollutants in WWTP-Effluents of Austria
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- Eunice Stevenson
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1 Pollutants in WWTP-Effluents of Austria Karlsruhe
2 Biological Water Quality in 1968
3 visible water pollution Source:
4 visible water pollution
5 visible water pollution
6 Measures Source: RHV Attersee, 1989
7 Measures Wastewater emission ordinances Austrian Water Act
8 Measures Source: RHV Attersee, 1989 Source: BMLFUW 2010, Austrian Situation Report 91/271/EEC
9 UWWTPs in Austria: size classes (p.e.) number of UWWTPs Capacity (p.e.) % % % % % % > % % Source: BMLFUW 2010, Austrian Situation Report 91/271/EEC 9
10 mg/m³ Biological Water Quality in Total Phosphorus in Lake Constance (Upper Lake)
11 Implementation of WFD in Austria WFD Annex II 1.4: Collection and maintainance of information about significant anthropogenic pressures Austrian Water Act, 59a: Electronic register of pressures and impacts Austrian ordinance for emissions register - surface water bodies (EMREG-SW) EQS - Ordinance - Surface water Chemistry (2006) (72 Substances and groups of substances) (72 Substances and groups of substances) Emissions from UWWTPs???? 11
12 Project: Emissions of organic and anorganic substances from UWWTPs Investigation of > 100 single substances in UWWTP s Categorisation and selection of UWWTPs 2 Step approach for defining the significant substances for UWWTPs for the Austrian Emission Register (EMREG-SW) Fate of selected substances in UWWTPs ( Balance) 12
13 Priority Substances 13 priority hazardous substances 20 priority substances Anthracen Alachlor Bromierte Diphenylether (PBDE) Atrazin Cadmium und Cadmiumverbindungen Benzol C10-13-Chloralkane Chlorfenvinphos Endosulfan Chlorpyrifos Hexachlorbenzol 1,2-Dichlorethan Hexachlorbutadien Dichlormethan Hexachlorcyclohexan Di(2-ethylhexyl)phthalat (DEHP) Quecksilber und Quecksilberverbindungen Diuron Nonylphenole (4-Nonylphenol) Fluoranthen Pentachlorbenzol Isoproturon Polyzyklische aromatische Kohlenwasserstoffe Blei und Bleiverbindungen Benzo(a)pyren Naphtalin Benzo(b)fluoranthen Nickel und Nickelverbindungen Benzo(k)fluoranthen Octylphenol Benzo(g,h,i)perylen Pentachlorophenol Indeno(1,2,3-cd)pyren Simazin Tributylzinnverbindungen (Tributylzinn-Kation) Trichlorobenzole Trichlormethan (Chloroform) Trifluralin priority hazardous substance cessation or phasing out of discharges, emissions and losses priority substances Reduction of discharges, emission and losses of substances 13
14 Other Substances 43 national and EU regulated substances and groups of substances Aldrin* 2,5-Dichlorophenol Pentachlornitrobenzene Ammonia 1,3 Dichloro-2-propanol Phosalon AOX Ethylendiaminetetraacetic acid EDTA Sebuthylazin Benzidine Endrin* Tetrachlorethen* Benzyl chloride Ethylbenzene Tetrachlormethan* Bisphenol-A Fluorid Trichlorethen* Chlordane Heptachlor Trichlorfon Chloroacetic acid Isodrin* Xylene Cyanides, free Isopropylbenzene Arsenic p-p -DDT* Linear Alkylbenzenesulfonates LAS Chromium DDT total* Mevinphos Copper Dibutyltin compounds Nitrit Selenium Dieldrin* Nitrilotriacetic acid NTA Silver 1,2-Dichloroethene Omethoat Zinc 2,4-Dichlorophenol * EU regulated Priority and other substances/group of substances > 100 single substances 14
15 Modul 1 UWWTP Categorisation and selection Categorisation criteria: Treatment Capacity Indirect dischargers (industrial influenc) o 5000 p.e. o p.e. o > p.e. o < 25% (mainly household ww) o 25%-75% (urban ww) o >75% (industrial dominated ww) 15 UWWTPs (35 % of installed capacity) 15
16 Modul 1 Sampling and chemical analytic of influent and effluent of the UWWTPs Literature study Significance criteria for identifying remaining substances for Modul 2 Maximum of the 15 effluent values is >EQS/2 16
17 Results Modul 1 Identification of substances in Modul 1 and basis for further investigation under Modul 2 Priority Substances polybrominated diphenyl ethers (PBDE) cadmium di(ethyl-hydroxyl)phthalate (DEHP) diurone nonylphenol mercury nickel tributyltin compounds National relevant Substances AOX EDTA NTA sebuthylazin trichlorfon copper selenium zinc 17
18 Modul 2 9 UWWTPs (~30 % of installed capacity) UWWTP effluents analysed 5 times in 2-month step Balance of 2 UWWTPs over 10 days (influent, effluent, sewage sludge) Additional analyses of pesticides Evaluation of the results Relevance criteria 1) Mean concentration of all effluent data from Modul 1 and 2 above EQS/2 2) Mean effluent concentration of at least of one UWWTP of Modul 2 greater then the EQS 18
19 Results Modul 2 Priority Substances o Relevance criteria 1): Mean concentration of all effluent values > EQS/2 PBDE, Cadmium, Nonylphenole and TBT comp Konzentration [µg/l] ,1 0,01 0,001 Konzentration/UQN [-] 1 0,1 0,0001 Summe PBDE Cadmium Quecksilber Nonylphenole Tributylzinnverbindungen DEHP Diuron Nickel 0,01 Summe PBDE Cadmium Quecksilber Nonylphenole Tributylzinnverb. DEHP Diuron Nickel 19
20 Results Modul 2 Priority Substances o Relevance criteria 2): Mean concentration of one UWWTP > EQS PBDE, Nonylphenole, Diuron and TBT comp. Konzentration/UQN [-] 5,00 4,00 3,00 2,00 1,00 0,75 0,50 0,25 PBDE Cadmium Nonylphenole Tributylzinn DEHP Diuron Nickel 0,00 ARA 1 ARA 2 ARA 3 ARA 4 ARA 5 ARA 6 ARA 7 ARA 8 ARA 9 20
21 Results Modul 2 other substances o Relevance criteria 1): Mean concentration of all effluent values > EQS/2 AOX, EDTA, NTA, (Trichlorfon), Copper, Selen und Zinc Konzentration [µg/l] Konzentration/UQN [-] AOX EDTA NTA Sebuthylazin Trichlorfon Kupfer Selen Zink 0,1 AOX EDTA NTA Sebuthylazin Trichlorfon Kupfer Selen Zink 21
22 Results Modul 2 other substances o Relevance criteria 2): Mean concentration of one UWWTP > EQS AOX, EDTA, NTA und Selen 20,00 Konzentration/UQN [-] 15,00 10,00 5,00 2,00 1,75 1,50 1,25 1,00 0,75 0,50 0,25 0,00 ARA 1 ARA 2 ARA 3 ARA 4 ARA 5 ARA 6 ARA 7 ARA 8 ARA 9 AOX EDTA NTA Selen 22
23 Results Modul 2 other substances o Relevance criteria 2): Mean concentration of one UWWTP > EQS Copper and Zinc Konzentration/UQN [-] 20,0 15,0 10,0 5,0 2,0 1,5 1,0 0,5 Kupfer Zink Kupfer und Zink 0,0 ARA 1 ARA 2 ARA 3 ARA 4 ARA 5 ARA 6 ARA 7 ARA 8 ARA 9 23
24 Results Modul 1 and 2 Relevant substances discharged from UWWTPs Priority Substances Polybromierte Diphenylether Cadmium Diurone Nonylphenole Tributyltin comp. Other substances AOX EDTA NTA Copper Selenium Zinc EMREG-SW relevant PS 24
25 Austrian Emission register on surface water bodies from point sources 25
26 Austrian Emission register on surface water bodies from point sources (EMREG SW) Standort Standort RPF Bes RPF Bes Direkteinleitung Anlage Emission / Teilstrom ELP Anlage Emission / Teilstrom ELP Direkteinleitung Standort RPF Bes Standort Anlage Emission / Teilstrom ELP RPF Bes Indirekteinleitung RPF Operator Bes Permit BE_EMREG-SW Facility ELP Discharge poin Mst Monitoring site Anlage Emission / Teilstrom ELP Direkteinleitung Messstelle
27 Austrian Emission register on surface water bodies from point sources Since 2009 operational Data covered: general master data, (operator, location of facility, ) Water management master data (discharge point, receiving water body, permit data, ) Annual Emission data (loads [kg/a], volume, ) 6-year reporting cycle 27
28 EMREG-SW relevant Summary 33/43 priority and other substances and groups of substances (> 100 single substances) 8/8 after Modul 1 4(5)/6 Cadmium after Modul 2 Diuron Nonylphenole Tributyltin comp. (PBDE) AOX EDTA NTA Copper Selen Zinc 28
29 invisible water pollution Example: Tributyltin compounds EQS = 0,2 ng/l Lake Attersee Volume: m³ Area: 47 km² ca.80 dag Quelle:
30 30
31 Thank you for your attention DI Georg Windhofer /3491 Dr. Manfred Clara /5612 Umweltbundesamt 31
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