An Overview of HydroGEN: A DOE Energy Materials Network, Aimed at Accelerating the R&D of Advanced Water Splitting Materials (AWSM)
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1 An Overview of HydroGEN: A DOE Energy Materials Network, Aimed at Accelerating the R&D of Advanced Water Splitting Materials (AWSM) H.N. Dinh, E.L. Miller, K. Randolph, A. Weber, A. McDaniel, R. Boardman, T. Ogitsu, and H. Colon-Mercado Date: 11/8/2017 Venue: Fuel Cell Seminar, Long Beach, CA Renewable Hydrogen Pathways Session Website:
2 Energy Materials Network (EMN) HydroGEN: Advanced Water Splitting Materials 2
3 Current EMN Consortia Overview Caloric materials for efficient cooling and heat pumping technologies. Catalytic materials for commercial bioenergy applications Durable module materials that reduce the levelized cost of energy of photovoltaic systems. Lightweight materials for automotive manufacturing. Platinum group metal-free catalysts for automotive fuel cells Hydrogen storage materials by providing capabilities and foundational understanding. Advanced water splitting technologies for clean, sustainable hydrogen production. HydroGEN: Advanced Water Splitting Materials 3
4 Goal: Widespread H 2 Production & Delivery Diverse Sources worldwide ~65M metric ton* Diverse Applications Growing industrial demand for H 2 >$100B global market and expanding Hydrogen enables domestic energy & environmental security, with large-scale market potential & with job creation and economic growth opportunities HydroGEN: Advanced Water Splitting Materials 4
5 HydroGEN Consortium Launch From drawing-board to consortium full deployment in 6 months! Visit the HydroGEN website at HydroGEN: Advanced Water Splitting Materials 5
6 HydroGEN: Advanced Water-Splitting Materials (AWSM) Consortium Accelerating discovery & development of innovative materials critical to advanced water splitting technologies for sustainable H 2 production, including: Photoelectrochemical (PEC) H H Solar Thermochemical (STCH) Hydrogen Water Low- and High-Temperature Advanced Electrolysis (LTE & HTE) Website: HydroGEN: Advanced Water Splitting Materials 6
7 Cross-Cutting Multiple Advanced Water Splitting Material (AWSM) Technologies Polymer Electrolyte Membrane Electrolysis (LTE) ee HH 22 HH 22 OO ee OO 22 Solid Oxide Electrolysis (HTE) H 2 O Sweep Gas Power Supply 2e - HH 22 OO + 22ee HH 22 + OO 22 Cathode (-) Solid oxide electrolyte OO 22 OO 22 Anode (+) OO ee H 2 1 / 2 O 2 Sweep Gas Solar Thermochemical (STCH) Photoelectrochemical (PEC) Hybrid Sulfur Cycle (HT) Hybrid = Electrolysis + STCH HydroGEN: Advanced Water Splitting Materials 7
8 Cross-Cutting Technologies and Collaboration Can Enable Reduction in H 2 Production Cost RD&D from different water splitting pathways is critical to reducing renewable H 2 production cost Production target <$2/gge H 2 Cost at Pump <$4/gge <$7/gge (early market) HydroGEN: Advanced Water Splitting Materials 8
9 Collaborations: HydroGEN Steering Committee Huyen Dinh (Director) Adam Weber (Deputy Director) Anthony McDaniel (Deputy Director) Richard Boardman Tadashi Ogitsu Héctor Colón-Mercado Eric Miller and Katie Randolph, FCTO HydroGEN: Advanced Water Splitting Materials 9
10 HydroGEN: Advanced Water-Splitting Materials (AWSM) Consortium Comprising more that 80 unique, world-class capabilities/expertise in: Materials Theory/Computation Advanced Materials Synthesis Characterization & Analytics LLNL NREL SNL SNL LLNL Bulk & interfacial models of aqueous electrolytes LAMMPS classic molecular dynamics modeling relevant to H 2 O splitting High-throughput spray pyrolysis system for electrode fabrication Conformal ultrathin TiO 2 ALD coating on bulk nanoporous gold Stagnation flow reactor to evaluate kinetics of redox material at high-t INL TAP reactor for extracting quantitative kinetic data Cross technology collaboration opportunities HydroGEN: Advanced Water Splitting Website: Materials 10
11 HydroGEN Website Enhanced Capability Search HydroGEN: Advanced Water Splitting Materials 11
12 HydroGEN Data Hub: Making digital data accessible HydroGEN Data Hub Home Page ( HydroGEN: Advanced Water Splitting Materials 12
13 Technology Transfer Activities Non-Disclosure Agreement (NDA) Streamlined Access Information Disclosure Intellectual Property Management Plan (IPMP) IP Protection Materials Transfer Agreement (MTA) Freedom to Operate Cooperative Research and Development Agreement (CRADA) Collaboration (nearly complete) Developed a catalog of pre-approved, mutual agreements between all consortium partners Facilitating rapid IP, NDA, and contract agreements HydroGEN: Advanced Water Splitting Materials 13
14 High Impact Publication Steering Committee Member (Tadashi) owns a FCEV and chooses a unique license plate HydroGEN: Advanced Water Splitting Materials 14
15 High Impact Publications & Patents World-record Photoelectrolysis Efficiency with Inverted Metamorphic Multi-junction Semiconductors Mass-spectrometer based Faradaic efficiency system Protected Layer to Enhance Durability Filed provisional patent on PASSIVATING WINDOW AND CAPPING LAYER FOR PHOTOELECTROCHEMICAL CELLS. on August 16, 2016 at the United States Patent & Trademark Office (USPTO) and has received Application No. 62/375,718. Filed a non-provisional patent on Devices and Methods for Photoelectrochemical water splitting March 23 rd, 2016 based on our IMM for high efficiency work. United States Patent Application Awaiting examination. High Impact Publications and Patent Applications HydroGEN: Advanced Water Splitting Materials 15
16 NEW HydroGEN Seedling Project 19 Proposals Selected, Negotiated, and Awarded 44 unique capabilities being utilized across 6 core labs Advance Electrolysis (8) LTE (5) HTE (3) PEC (5) STCH (5) Benchmarking & Protocols (1) 2-Step MO x (4) Hybrid cycle (1) To learn more, check HydroGEN website or contact huyen.dinh@nrel.gov HydroGEN: Advanced Water Splitting Materials 16
17 HydroGEN EMN Website: Core Labs Comprising more than 80 unique, world-class capabilities/expertise in materials theory/computation, synthesis, and characterization & analysis: Materials Theory/Computation Advanced Materials Synthesis Characterization & Analysis LLNL NREL SNL SNL Bulk and interfacial models of aqueous electrolytes High-throughput spray pyrolysis system for electrode fabrication Stagnation flow reactor to evaluate kinetics of redox material at high-t INL LAMMPS classic molecular dynamics modeling relevant to H 2 O splitting Conformal ultrathin TiO 2 ALD coating on bulk nanoporous gold TAP reactor for extracting quantitative kinetic data HydroGEN is enabling innovative, world-class research of water-splitting materials and catalysts. HydroGEN: Advanced Water Splitting Materials 17
18 Acknowledgements DOE EERE Fuel Cell Technology Office Team Eric Miller and Katie Randolph, (Leads) David Peterson James Vickers Maxim Lyubovsky Kim Cierpik-Gold
19 Acknowledgements NREL Team Huyen Dinh, Lead Principal Investigators: Shaun Alia Mowafak Al-Jassim Guido Bender Jeff Blackburn Kai Zhu Todd Deutsch Daniel Friedman David Ginley Kevin Harrison Steven Harvey Stephan Lany Zhiwen Ma Kristin Munch Judy Netter John Perkins Bryan Pivovar Matthew Reese Genevieve Saur Glenn Teeter Michael Ulsh Judith Vidal Andriy Zakutayev LBNL Team Adam Weber, Lead Principal Investigators: Nemanja Danilovic Ian Sharp Peter Agbo David Larson Lin-Wang Wang Walter Drisdell Mike Tucker SRNL Team Francesca Toma Miquel Salmeron Ethan Crumlin Jeffrey Greenblat Ahmet Kusoglu Frances Houle David Prendergast Hector Colón-Mercado, Lead Principal Investigators: Maximilian Gorensek Brenda Garcia-Diaz
20 Acknowledgements LLNL Team Tadashi Ogitsu, Lead Principal Investigators: SNL Team Anthony McDaniel, Lead Principal Investigators: Mark Allendorf Eric Coker Bert Debusschere Farid El Gabaly Lindsay Erickson Ivan Ermanoski James Foulk Cy Fujimoto Fernando Garzon Ethan Hecht Reese Jones Bryan Kaehr David Littlewood John Mitchell Jeff Nelson Peter Schultz Randy Schunk Subhash Shinde Josh Sugar Alec Talin Alan Wright Sarah Baker Monika Biener Alfredo Correa Tedesco Thomas Yong-Jin Han Tae Wook Heo Jonathan Lee Miguel Morales-Silva Christine Orme INL Team Richard Boardman, Lead Principal Investigators: James O Brien Dong Ding Rebecca Fushimi Dan Ginosar Tuan Anh Pham Christopher Spadaccini Tony Van Buuren Joel Varley Trevor Willey Brandon Wood Marcus Worsley Ting He Gabriel Ilevbare Soe Lwin Carl Stoots
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